Full-scale production of plutonium-238 still years away

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The United States has begun manufacturing nuclear spacecraft fuel for the first time in a generation, but full production of the stuff is still seven years or so away.

In December, officials at the Department of Energy’s (DOE) Oak Ridge National Laboratory in Tennessee announced that researchers at the site had generated a 1.8-ounce (50 grams) sample of plutonium-238, the fuel that powers deep-space missions such as NASA’s New Horizons Pluto probe and Cassini Saturn orbiter.

The milestone marked the first domestic production of Pu-238 since the Savannah River Site in South Carolina, another DOE facility, stopped making the fuel in the late 1980s. But Oak Ridge is still at the proof-of-concept stage in the restart, and it will therefore be a few years before the lab begins churning out large amounts of Pu-238, officials said.

“What we’re shooting for is to get to an interim production level of around 400 to 500 grams [14 to 18 ounces] per year in 2019, and then full-scale, a kilogram and a half [3.3 lbs.] — if everything goes right — in 2023,” Bob Wham, the Pu-238 project lead in the Nuclear Security and Isotope Technology division at Oak Ridge, said last month during a presentation with NASA’s Future In-Space Operations (FISO) working group.

Deep-space power
Plutonium-238 is the key ingredient in radioisotope thermoelectric generators (RTGs), which convert into electricity the substantial heat emitted by the radioactive Pu-238 when it naturally decays into uranium-234.

For more than 50 years, RTGs have been the power source of choice for missions that travel far enough from the sun to make solar panels impractical. Some famous examples include NASA’s twin Voyager 1 and Voyager 2 probes, which launched in 1977 and have recently been exploring the solar system’s extreme outer reaches. (Voyager 1 actually reached interstellar space in 2012.)

From the early 1960s through the late 1980s, the Pu-238 needed for such missions was made at the Savannah River Site, as an offshoot of the facility’s weapons-production program. (Plutonium-238 is not used to make nuclear weapons, but its close cousin, plutonium-239 — which harbors one more neutron in its nucleus than does Pu-238 — is a common bomb-making material.)

Savannah River stopped making Pu-238 in 1988, as the Cold War wound down. In 1992, the United States started buying the stuff from Russia, but the last such foreign shipment was received in 2010. Since then, U.S. stores of Pu-238 have been dwindling.

The country currently has just 77 lbs. (35 kg) of the spacecraft fuel left, and only about half of that stockpile is suitable for power production as-is (though the rest could conceivably be made usable by blending it with newly produced Pu-238, DOE officials have said.)

RTGs like the one powering NASA’s Mars rover Curiosity use 10.6 lbs. (4.8 kg) of Pu-238, so right now there’s enough of the stuff to power perhaps three more such deep-space missions, DOE officials have said.

The activities underway at Oak Ridge are therefore designed to avert a possible shortage and keep NASA spacecraft cruising through deep space for decades to come. NASA officials have said 3.3 lbs. (1.5 kg) of new Pu-238 per year should suffice to accommodate the agency’s needs.

Making nuclear fuel
As you might expect, the production of Pu-238 is complicated. First, the Oak Ridge team receives shipments of radioactive neptunium-237 from Idaho National Laboratory (INL), another DOE facility.

Engineers then process the neptunium into “targets,” which are blasted with beams of neutrons in one of two nuclear reactors at Oak Ridge, Wham said. This creates Pu-238, which is then chemically processed and shipped to a third DOE site, Los Alamos National Laboratory in New Mexico.

Los Alamos personnel further process the stuff, creating encapsulated “pellets” that are then shipped to INL for integration into RTGs. The power systems are tested at the Idaho site, and, if all goes well, they are then shipped to NASA’s Kennedy Space Center in Florida to be prepared for launch.

The restart of Pu-238 production hasn’t made it to these latter few steps, however; Oak Ridge is still figuring out the best way to manufacture and process the plutonium. The team can’t simply copy what was done at Savannah River during the Cold War, because the facilities involved are quite different.

For example, the nuclear reactors that Oak Ridge has available are quite small, about as wide as a 55-gallon (208 liters) drum, Wham said. (Use of the Savannah facilities is not an option, he added; the Savannah reactors that once produced Pu-238 have been shut down.)

The restart team is also trying out a new processing technique, one that relies on solvent extraction as opposed to exchange columns, Wham said. Savannah River identified solvent extraction as a good way to reduce both costs and waste back in 1977 but never adopted the technique, he added.

“At the time, it just wasn’t that important to them to do that, because this was a small part of the overall mission to produce plutonium for weapons,” Wham said during the FISO talk. “We’ve adopted that [solvent extraction] as being kind of our baseline, because we want to reduce operating costs, and reduce the waste.”

The ball is rolling
The wheels of the Pu-238 restart are turning. Oak Ridge has already made some plutonium, after all, and the lab shipped two small samples (0.2 ounces, or 5 grams each) of the stuff to Los Alamos earlier this year, Wham said.

It will take considerable time and effort to validate all of the procedures involved and get fully up to speed. For example, the team is currently testing a way to increase yields and significantly reduce the number of neptunium-237 “targets” needed, by using pure neptunium-oxide pellets clad in zirconium alloy as opposed to a neptunium oxide-aluminum mix.

“It’ll probably be another year and a half before we have sufficient information to make a decision on whether this is worth pursuing and scaling up into target design,” Wham said.

But the team should be able to start producing the NASA-requested 3.3 lbs. (1.5 kg) of Pu-238 per year by 2023, if everything goes well, Wham said. And that production should continue indefinitely, provided the will and the funding don’t disappear, he added; the nation stockpiled hundreds of kilograms of neptunium-237 during the Cold War.

“We could make new plutonium-238 for a very long time with the current amount of material that we have,” Wham said.

This story originally appeared on Space.com. Used with permission.